Cliff Robertson

Cole Younger

Robert Duvall

Jesse James

Luke Askew

Jim Younger

R.G. Armstrong

Clell Miller

Dana Elcar

Allen

Donald Moffat

Manning

John Pearce

Frank James

Matt Clark

Bob Younger

Wayne Sutherlin

Charley Pitts

Robert H. Harris

Wilcox

Jack Manning

Heywood

Elisha Cook Jr.

Bunker (as Elisha Cook)

Royal Dano

Gustavson

Mary-Robin Redd

Kate

William Callaway

Calliopist

Philip Kaufman